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Richmond Park is a 2,360 acre (3.69 sq mi) park within London. It is the largest of the Royal Parks in London and Britain's second largest urban walled park after Sutton Park, Birmingham. It is close to Richmond, Ham, Kingston upon Thames, Wimbledon, Roehampton and East Sheen. The park is famous for its red and fallow deer, which number over six hundred. The park is a National Nature Reserve. There is access to the park through several gates and many footpaths cross the park.
Website & map: Link
Wikipedia: Link

The Capital Ring is a surprisingly green route that encircles London. Distance is 78miles; it threads together parks and open spaces, mostly following pleasant residential roads in between. The route is an initiative of the London Walking Forum. The route is very well signed, with a Big Ben logo TQ1678 : Three walk logos, Gallows Bridge. The route is a walker’s equivalent of the North and South Circular roads. Link